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许鹏飞

【来源:功能有机分子化学国家重点实验室 | 发布日期: | 作者: 】     【选择字号:
许鹏飞
博士、教授
电话:+86-931-8912281
传真:+86-931-8915557
邮箱:xupf@lzu.edu.cn
 
教育背景、工作经历
2015-至今           兰州大学萃英学院执行院长
2009-2015          兰州大学教务处处长
2003-至今           兰州大学化学化工学院、功能有机分子化学国家重点实验室,教授
2003-2004          日本名古屋大学物质材料科学国际研究中心(K. Tatsumi合作教授), 访问教授
1999-2001          台湾中兴大学,博士后(陆大荣教授)
1996-1998          兰州大学,理学博士(张自义教授)
1992-1994          兰州大学,理学硕士(吴绍祖教授)
1983-1987          兰州大学,化学系有机化学专业,理学学士(李瑜教授)
 
荣誉奖励
2016                   兰州大学国华杰出学者奖
2014                   全国宝钢优秀教师奖
2014                   甘肃省科技进步一等奖(第一完成人)
2013                   兰州大学 “师德标兵”,甘肃省 “陇原师德先进个人” 称号
2012                   金川集团科技进步一等奖,国务院政府特殊津贴
2010                   甘肃省自然科学一等奖(第一完成人)
2009                   入选甘肃省领军人才,Thieme Chemistry Journal Award
2005                   入选教育部 “新世纪优秀人才支持计划”、甘肃省 “555” 创新人才
2002                   第九届甘肃省青年教师成才奖,甘肃省科技进步三等奖两项
 
研究兴趣
1) α-氨基酸的不对称合成及方法研究
2) 有机小分子催化的不对称串联反应的研究
3) 天然产物结构导向的有机小分子催化反应的研究
4) 可见光催化的有机反应研究
5) 新型可见光催化剂的设计与应用
6) 新型浮选剂的研发
 
代表成果
1.   “Asymmetric Catalytic Cascade Reactions for Constructing Diverse Scaffolds and Complex Molecules”. Wang, Y.; Lu, H.; Xu, P.-F. * Acc. Chem. Res. 2015, 48, 1832.
2.   “Synthesis of a-Amino Acids Based on Chiral Tricycloiminolactone Derived from Natural (+)-Camphor”. Luo, Y.-C.; Zhang, H.-H.; Wang, Y.; Xu, P.-F.* Acc. Chem. Res. 2010, 43, 1317.
3.   “Rationally Designed Multifunctional Supramolecular Iminium Catalysis: Direct Vinylogous Michael Addition of Unmodified Linear Dienol Substrates”. Gu, Y.; Wang, Y.; Yu, T.-Y.; Liang, Y.-M.;* Xu, P.-F.* Angew. Chem., Int. Ed. 2014, 53, 14128.
4.   “Hydrogen-Bond-Mediated Supramolecular Iminium Ion Catalysis”. Wang, Y.; Yu, T.-Y.; Zhang, H.-B.; Luo, Y.-C; Xu, P.-F.* Angew. Chem., Int. Ed. 2012, 51, 12339.
5.   “Asymmetric Organocatalytic Relay Cascades: Catalyst-Controlled Stereoisomer Selection in the Synthesis of Functionalized Cyclohexanes”. Wang, Y.; Han, R.-G.; Zhao, Y.-L.; Yang, S.; Dixon, D. J.; Xu, P.-F.* Angew. Chem., Int. Ed. 2009, 48, 9834.
6.   “Catalytic Cascade Reactions”. Xu, P.-F., Wang, W., Eds.; John Wiley & Sons: Canada, 2014.
7.   “Iridium(1+), Bis(acetonitrile)bis[2-[5-(1,1-dimethylethyl)-2-benzothiazolyl-kN3]phenyl-kC]-,(OC-6-13 -Λ) Hexafluorophosphate(1-) (1:1)”. Xu, G.-Q.; Liang, H.; Xu, P.-F.* Encyclopedia of reagents for Organic Synthesis [Online], John Wiley & Sons Ltd., 2017.
8.   “N-Heterocyclic Carbene-Catalyzed Atom-Economical and Enantioselective Construction of the C-S Bond: Asymmetric Synthesis of Functionalized Thiochromans”. Lu, H.; Zhang, J.-L.; Liu, J.-Y.; Li, H.-Y.; Xu, P.-F.* ACS Catal. 2017, 7, 7797.
9.   “3,4,5-Trimethylphenol and Lewis Acid Dual-Catalyzed Cascade Ring-Opening/Cyclization: Direct Synthesis of Naphthalenes”. Ma, H.; Hu, X.-Q.;* Luo, Y.-C.; Xu, P.-F.* Org. Lett. 2017, 19, 6666.
10. “Visible-Light-Induced Aza-Pinacol Rearrangement: Ring Expansion of Alkylidenecyclopropanes”. Liu, W.-D.; Xu, G.-Q.; Hu, X.-Q.; Xu, P.-F.* Org. Lett. 2017, 19, 6291.
11.  “Highly Enantioselective Construction of Hajos-Wiechert Ketone Skeletons via an Organocatalytic Vinylogous Michael/Stetter Relay Sequence”. Jia, Z.-L.; Wang, Y.; Zhao, C.-G.; Zhang, X.-H.; Xu, P.-F.* Org. Lett. 2017, 19, 2130.
12.  “Quaternary Carbon Center Forming Formal [3+3] Cycloaddition Reaction via Bifunctional Catalysis: Asymmetric Synthesis of Spirocyclohexene Pyrazolones”. Liu, J.-Y.; Zhao, J.; Zhang, J.-L.; Xu, P.-F.* Org. Lett. 2017, 19, 1846.
13.  “Synthesis of Fused Pyran Derivatives via Visible-Light-Induced Cascade Cyclization of 1,7-Enynes with Acyl Chlorides”. Li, C.-G.; Xu, G.-Q; Xu, P.-F.* Org. Lett. 2017, 19, 512.
14.  “Rh(II) Catalyzed High Order Cycloadditions of 8-Azaheptafulvenes with N-Sulfonyl 1,2,3-Triazloes or α-Oxo Diazocompounds”. Chen, W.; Bai, Y.-L.; Luo, Y.-C.; Xu, P.-F.* Org. Lett. 2017, 19, 364.
15.  “Lewis acid catalyzed diastereoselective [3+4]-annulation of donor-acceptor cyclopropanes with anthranils: synthesis of tetrahydro-1-benzazepine derivatives”. Wang, Z.-H.; Zhang, H.-H.;* Wang, D.-M.; Xu, P.-F.; Luo, Y.-C.* Chem.Commun. 2017, 53, 8521.
16.  “Kinetic resolution via supramolecular iminium catalysis: multiactivation enables the asymmetric synthesis of beta-aryl substituted aldehydes and densely functionalized cyclohexanes”. Jia, Z.-L.; Wang, Y.; Xu, G.-Q.; Xu, P.-F.* Chem.Commun. 2017, 53, 4938.
17.  “Metal-Free, Visible-Light-Promoted Synthesis of 3-Phosphorylated Coumarins via Radical C-P/C-C Bond Formation”. Liu, D.; Chen, J.-Q.; Wang, X.-Z.; Xu, P.-F.* Adv. Synth. Catal. 2017, 359, 2773.
18.     “Aroyl chlorides as novel acyl radical precursors via visible-light photoredox catalysis”. Xu, S.-M.; Chen, J.-Q.; Liu, D.; Bao, Y.; Liang, Y.-M.; Xu, P.-F.* Org. Chem. Front. 2017, 4, 1331.
19.  “Direct Noncovalent Activation of a,b-Unsaturated Aldehydes for the Stereodivergent Synthesis of Substituted Cyclohexenes”. Xie, J.-K.; Wang, Y.; Lin, J.-B.; Ren, X.-R.; Xu, P.-F.* Chem. Eur. J. 2017, 23, 6752.
20.  “Direct DecarboxylativeDecarbonylative Alkylation of a-Oxo Acids with Electrophilic Olefins via Visible-Light Photoredox Catalysis”. Chen, J.-Q.; Chang, R. Wei, Y.-L.; Mo, J.-N.; Wang, Z.-Y.; Xu, P.-F.* J. Org. Chem. 2018, 83, 253.
21.  “PPh3 Mediated Reductive Annulation Reaction between Isatins and Electron Deficient Dienes to Construct Spirooxindole Compounds”. Zhang, L.; Lu, H.; Xu, G.-Q.; Wang, Z.-Y.; Xu, P.-F.* J. Org. Chem. 2017, 82, 5782.
22.  “Sc(OTf)3 Catalyzed [4 + 2]-Annulation Reaction between Electron-Rich Phenols and Donor–Acceptor Cyclopropanes: Synthesis of Polysubstituted Dihydronaphthols”. Luo, Y.-C.; Ma, H.; Hu, X.-Q.; Xu, P.-F.* J. Org. Chem. 2017, 82, 1013.
23.  “Photoredox-Induced Functionalization of Alkenes for the Synthesis of Substituted Imidazolines and Oxazolidines”. Chen, J.-Q.; Yu, W.-L.; Wei, Y.-L.; Li, T.-H.; Xu, P.-F.* J. Org. Chem. 2017, 82, 243.
24.  “Exploring the Reactivity of Nitro-Activated 1,3-Enynes in an Organocatalytic One-Pot, Three-Component Coupling Reaction: A Tandem Catalytic Approach to a Novel 3-Nitrochroman Scaffold”. Xiao, Y.; Lin, J.-B.; Zhao, Y.-N.; Liu, J.-Y.; Xu, P.-F.* Org. Lett. 2016, 18, 6276.
25.  “Dual C–H Functionalization of N-aryl Tetrahydroisoquinolines: A Highly Diastereoselective Synthesis of Dibenzo[a,f]quinolizines via Visible-Light Induced Oxidation and Inverse Electron-Demand Aza-Diels–Alder Reaction”. Xu, G.-Q.; Li, C.-G.; Liu, M.-Q.; Cao, J. Luo Y.-C.; Xu, P.-F.* Chem. Commun. 2016, 52, 1190.
26.  “Intramolecular 1,5-H Transfer Reaction of Aryl Iodides through Visible-Light Photoredox Catalysis: A Concise Method for the Synthesis of Natural Product Scaffolds”. Chen, J.-Q.; Wei, Y.-L.; Xu, G.-Q.; Liang, Y.-M.; Xu, P.-F.* Chem. Commun. 2016, 52, 6455.
27.   “Catalytic Enantioselective α-Fluorination of 2-Acyl Imidazoles via Iridium Complexes”. Xu, G.-Q.; Liang, H.; Fang, J.; Jia, Z.-L.; Chen, J.-Q.; Xu, P.-F.* Chem. Asian J. 2016. 11, 3355.
28.  “Hydrogen-Bonding Network Promoted [3+2] Cycloaddition: Asymmetric Catalytic Construction of Spiro-pseudoindoxyl Derivatives”. Zhang, L.-J.; Wang, Y.; Hu, X.-Q.; Xu, P.-F.* Chem. Asian J. 2016. 11,834.
29.   “Synthesis of Spirocyclic Oxindole Dihydrothiophenes by DBU-Catalyzed [3 + 2] Annulation of Morita–Baylis–Hillman Carbonates with Isothiocyanates”. Zhao, Y.-Y.; Zhao, S.; Xie, J.-K.; Hu, X.-Q.; Xu, P.-F.* J. Org. Chem. 2016, 81, 10532.
30.  “Catalyst-Free Chemoselective Synthesis of 3,4-Dihydroquinazoline-2-thiones and 2-Imino[1,3] -benzothiazines”. Xie, T.; Xiao, Y.; Zhao, S.; Hu, X.-Q.; Xu, P.-F.* J. Org. Chem. 2016, 81, 10499.
31.  “PPh3O as an Activating Reagent for One-Pot Stereoselective Syntheses of Di- and Polybrominated Esters from Simple Aldehydes”. Yu, T.-Y.; Wei, H.; Luo, Y.-C.; Wang, Y.; Wang, Z.-Y.; Xu, P.-F.* J. Org. Chem. 2016, 81, 2730.
32.  “Direct Construction of Chiral Quaternary Dihydropyranones through Highly Enantioselective Organocatalytic Hetero-Diels–Alder reactions of Olefinic Azlactones”. Gao, T.-P.; Liu, D.; Lin, J.-B.; Hu, X.-Q.; Wang, Z.-Y.; Xu, P.-F.* Org. Chem. Front. 2016, 3, 598.
 

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