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许鹏飞

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许鹏飞

博士、教授

电话:+86-931-8912281

传真:+86-931-8915557

邮箱: xupf@lzu.edu.cn

•教育背景、工作经历

       2019-至今           兰州大学校长助理

2018-至今            科学技术发展研究院执行院长

2015-2018           兰州大学萃英学院执行院长

2009-2015           兰州大学教务处处长

2003-至今            兰州大学化学化工学院、功能有机分子化学国家重点实验室,教授

2003-2004           日本名古屋大学物质材料科学国际研究中心(K. Tatsumi合作教授), 访问教授

1999-2001           台湾中兴大学,博士后(陆大荣教授)

1996-1998           兰州大学,理学博士(张自义教授)

1992-1994           兰州大学,理学硕士(吴绍祖教授)

1983-1987           兰州大学,化学系有机化学专业,理学学士(李瑜教授)

•荣誉奖励

       2019                  甘肃省自然科学一等奖(第一完成人);甘肃省拔尖人才

2016                   兰州大学国华杰出学者奖;

2014                   全国宝钢优秀教师奖;

2014                   甘肃省科技进步一等奖(第一完成人);

2013                   兰州大学“师德标兵”,甘肃省“陇原师德先进个人”称号;

2012                   金川集团科技进步一等奖,国务院政府特殊津贴;

2010                   甘肃省自然科学一等奖(第一完成人);

2009                   入选甘肃省领军人才,Thieme Chemistry Journal Award;

2005                  入选教育部“新世纪优秀人才支持计划”、甘肃省“555”创新人才;

2002                  第九届甘肃省青年教师成才奖,甘肃省科技进步三等奖两项。

•研究兴趣

1) α-氨基酸的不对称合成及方法研究;

2) 有机小分子催化的不对称串联反应的研究;

3) 天然产物结构导向的有机小分子催化反应的研究;

4) 可见光催化的有机反应研究;

5) 新型可见光催化剂的设计与应用;

6) 新型浮选剂的研发。

•代表成果           

1.“Highly Enantioselective Construction of Strained Spiro[2,3]hexanes via Michael-Ring Expansion-Cyclization Cascade Strategy”. Zhao, C.-G.; Z.-T. Feng; Xu, G.-Q; * Gao, A.; Chen, J.-W.; Wang, Z.-Y. and Xu, P.-F. * Angew. Chem. Int. Ed. 2020, DIO: 10.1002/anie.201912834.

2.“Dehydrogenative Silylation of Alkenes for the Synthesis of Substituted Allylsilanes by Photoredox, Hydrogen-Atom Transfer, and Cobalt Catalysis”. Yu, W.-L.; Luo, Y.-C.; Yan, L.; Liu, D.; Wang, Z.-Y.; Xu, P.-F.* Angew. Chem. Int. Ed. 2019, 58, 10941.

3.“Ni-Catalyzed 1,2-Acyl Migration Reactions Triggered by C–C Bond Activation of Ketones” Jiang, C.; Lu, H.; Xu, W.; Wu, J.; Yu, T.-Y.; Xu, P.-F.; Wei, H.;* ACS Catal. 2019, DOI: 10.1021/acscatal.9b04112

4.“Photocatalyzed Metal-Free Alkylheteroarylation of Unactivated Olefins via Direct Acidic C(sp3)−H Bond Activation”. Fang, J.; Dong, W.-L.; Xu, G.-Q. and Xu, P.-F.*, Org. Lett. 2019, 21, 4480−4485.

5.“Metal-Free Visible-Light-Induced Construction of Difluoro- Containing Dibenzazepines”. Liu, D.; Meng-Jie Jiao, Xing-Zhi Wang, and Xu, P.-F.* Org. Lett. 2019, 21, 4745.

6. An Atropo-enantioselective Synthesis of Benzo-Linked Axially Chiral Indoles via Hydrogen-Bond Catalysis, Liu, J.-Y.; Yang, X.-C.; Liu, Z.; Luo, Y.-C.; Lu, H.; Gu, Y.-C.; Fang, R.; Xu, P.-F. *, Org. Lett. 2019, 21, 5219.

7.“Aroylchlorination of 1,6-Dienes via a Photoredox Catalytic Atom-Transfer Radical Cyclization Process”. Zhao, Q.-S.; Xu, G.-Q.; Liang, H.; Wang, Z.-Y.; and Xu, P.-F.*  Org. Lett. 2019, 21, 8615.

8.“Synthesis of indolo[2,1-a]isoquinoline derivatives via visible-light-induced radical cascade cyclization reactions” Wei, Y.-L.; Chen, J.-Q.; Sun, B.; Xu, P.-F.* Chem. Commun. 2019, 55, 5922.

9.“Directed Decarbonylation of Unstrained Aryl Ketones via Nickel-Catalyzed C—C Bond Cleavage”. Zhao, T.-T.; Xu, W.-H.; Zheng, Z.-J.; Xu, P.-F.;* H. Wei* J. Am. Chem. Soc. 2018, 140, 586.

10.“Dual CSp3-H Bond Functionalization of N-Heterocycles via Visible-Light Photocatalyzed Dehydrogenation /[2+2] Cycloaddition Sequential Reaction”. Xu, G.-Q., Xu, J.-T., Feng, Z.-T., Liang, H., Wang, Z.-Y., Qin, Y.; Xu, P.-F.* Angew. Chem. Int. Ed. 2018, 57, 5110.

11.“Organocatalytic, Enantioselective Friedel−Crafts Reaction of Indoles in the Carbocyclic Ring and Electron-Rich Phenols”. Liu, J.-Y.; Yang, X.-C.; Lu, H.; Gu, Y.-C.; Xu, P.-F.* Org. Lett. 2018, 20, 2190.

12.“Photoredox-Induced Intramolecular 1,5‑H Transfer Reaction of Aryl Iodides for the Synthesis of Spirocyclic γ‑Lactams”. Chen, J.-Q.; Chang, R.; Lin, J.-B.; Luo, Y.-C.; Xu, P.-F.* Org. Lett. 2018, 20, 2395.

13.“Regiospecific Three-Component Aminofluorination of Olefins via Photoredox Catalysis”. Mo, J.-N.; Yu, W.-L.; Chen, J.-Q.; Hu, X.-Q.;* Xu, P.-F.* Org. Lett. 2018, 20, 4471.

14.“Design, Synthesis, and Application of Highly Reducing Organic Visible-Light Photocatalysts”. Liu, D.; Jiao, M.-J.; Feng, Z.-T.; Wang, X.-Z.; Xu, G.-Q.; Xu, P.-F.* Org. Lett. 2018, 20, 5700.

15.“Dearomative Dienolate-Mediated Catalysis: A Remote Activation Strategy for Asymmetric Functionalization of Benzylic C−H Bonds of Heteroaryl Aldehydes”. Wang, Y.; Lin, J.-B.; Xie, J.-K.; Lu, H.; Hu, X.-Q.;* Xu, P.-F.* Org. Lett. 2018, 20, 5835.

16.“Alkene functionalization for the stereospecific synthesis of substituted aziridines by visible-light photoredox catalysis”. Yu, W.-L.; Chen, J.-Q.; Wei, Y.-L.; Wang, Z.-Y.; Xu, P.-F.* Chem. Commun. 2018, 54, Advance Article, 1948.

17.“A new approach to access difluoroalkylated diarylmethanes via visible-light photocatalytic cross-coupling reactions”. Zhao, Y.-N.; Luo, Y.-C.; Wang Z.-Y.; Xu, P.-F.* Chem. Commun. 2018, 54, 3993.

18.“Synthesis of five-membered cyclic nitrones based on the Lewis acid-catalysed [3+2]-annulation reaction of donor–acceptor cyclopropanes with 1,4,2-dioxazoles”. Wang, Z.-H.; Zhang, H.-H.;* Xu, P.-F.; Luo, Y.-C.* Chem. Commun. 2018, 54, 10128.

19.“N‑Heterocyclic Carbene-Catalyzed Atom-Economical and Enantioselective Construction of the C−S Bond: Asymmetric Synthesis of Functionalized Thiochromans”. Lu, H.; Zhang, J.-L.; Liu, J.-Y.; Li, H.-Y.; Xu, P.-F.* ACS Catal. 2017, 7, 7797.

20.“3,4,5-Trimethylphenol and Lewis Acid Dual-Catalyzed Cascade Ring-Opening/Cyclization: Direct Synthesis of Naphthalenes”. Ma, H.; Hu, X.-Q.;* Luo, Y.-C.; Xu, P.-F.* Org. Lett. 2017, 19, 6666.

21.“Visible-Light-Induced Aza-Pinacol Rearrangement: Ring Expansion of Alkylidenecyclopropanes”. Liu, W.-D.; Xu, G.-Q.; Hu, X.-Q.; Xu, P.-F.* Org. Lett. 2017, 19, 6291.

22.“Highly Enantioselective Construction of Hajos-Wiechert Ketone Skeletons via an Organocatalytic Vinylogous Michael/Stetter Relay Sequence”. Jia, Z.-L.; Wang, Y.; Zhao, C.-G.; Zhang, X.-H.; Xu, P.-F.* Org. Lett. 2017, 19, 2130.

23.“Quaternary Carbon Center Forming Formal [3+3] Cycloaddition Reaction via Bifunctional Catalysis: Asymmetric Synthesis of Spirocyclohexene Pyrazolones”. Liu, J.-Y.; Zhao, J.; Zhang, J.-L.; Xu, P.-F.* Org. Lett. 2017, 19, 1846.

24.“Synthesis of Fused Pyran Derivatives via Visible-Light-Induced Cascade Cyclization of 1,7-Enynes with Acyl Chlorides”. Li, C.-G.; Xu, G.-Q; Xu, P.-F.* Org. Lett. 2017, 19, 512.

25.“Rh(II) Catalyzed High Order Cycloadditions of 8-Azaheptafulvenes with N-Sulfonyl 1,2,3-Triazloes or α-Oxo Diazocompounds”. Chen, W.; Bai, Y.-L.; Luo, Y.-C.; Xu, P.-F.* Org. Lett. 2017, 19, 364.

26.“Lewis acid catalyzed diastereoselective [3+4]-annulation of donor-acceptor cyclopropanes with anthranils: synthesis of tetrahydro-1-benzazepine derivatives”. Wang, Z.-H.; Zhang, H.-H.;* Wang, D.-M.; Xu, P.-F.; Luo, Y.-C.* Chem. Commun. 2017, 53, 8521.

27.“Kinetic resolution via supramolecular iminium catalysis: multiactivation enables the asymmetric synthesis of beta-aryl substituted aldehydes and densely functionalized cyclohexanes”. Jia, Z.-L.; Wang, Y.; Xu, G.-Q.; Xu, P.-F.* Chem. Commun. 2017, 53, 4938.

28.“Asymmetric Catalytic Cascade Reactions for Constructing Diverse Scaffolds and Complex Molecules”. Wang, Y.; Lu, H.; Xu, P.-F. * Acc. Chem. Res. 201548, 1832.

29.“Catalytic Cascade Reactions”. Xu, P.-F., Wang, W., Eds.; John Wiley & Sons: Canada, 2014.

30.“Rationally Designed Multifunctional Supramolecular Iminium Catalysis: Direct Vinylogous Michael Addition of Unmodified Linear Dienol Substrates”. Gu, Y.; Wang, Y.; Yu, T.-Y.; Liang, Y.-M.;* Xu, P.-F.* Angew. Chem., Int. Ed. 2014, 53, 14128.

31.“Hydrogen-Bond-Mediated Supramolecular Iminium Ion Catalysis”. Wang, Y.; Yu, T.-Y.; Zhang, H.-B.; Luo, Y.-C; Xu, P.-F.* Angew. Chem., Int. Ed. 2012, 51, 12339.

32.“Synthesis of a-Amino Acids Based on Chiral Tricycloiminolactone Derived from Natural (+)-Camphor”. Luo, Y.-C.; Zhang, H.-H.; Wang, Y.; Xu, P.-F.* Acc. Chem. Res. 2010, 43, 1317.

33.“Asymmetric Organocatalytic Relay Cascades: Catalyst-Controlled Stereoisomer Selection in the Synthesis of Functionalized Cyclohexanes”. Wang, Y.; Han, R.-G.; Zhao, Y.-L.; Yang, S.; Dixon, D. J.; Xu, P.-F.* Angew. Chem., Int. Ed. 2009, 48, 9834.

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